Dye lasers are utilized in a wide variety of scientific, commercial, and military applications, primarily due to their ability to provide continuous tuning across a broad spectral range covering the ultraviolet, visible, and near-infrared. dye lasers are notoriously inefficient, primarily due to inefficiencies of the lasers used to pump then (argon, doubled Nd:YAG, nitrogen, excimer, etc.) During our recently completed Phase I contract, we studied the possibility of directly pumping dye lasers using already existing efficient semiconductor diode lasers, resulting in an efficient dye laser system. In addition to proving the feasibility of the approach, we identified a number of promising candidate dye/diode systems. We propose, during the Phase II effort described in this proposal, to determine the lazing parameters of, and demonstrate assisted and direct diode-pumping of two dyes in the continuous wave (CW) mode. In addition, we propose to extend the operation of at least one diode-pumped dye lapser to the pulsed mode. Significant increases in the efficiency of dye lasers will be demonstrated during the proposed program.